Description
We develop a general theory of high-harmonic generation (HHG) in solid-state systems, based on a weak-correlation expansion of photonic and matter degrees of freedom. Unlike standard HHG theories, which treat light-matter dynamics through the Schr¨odinger equation, our approach employs density-matrix evolution, naturally capturing the mixed-state character of both the field and the matter - a critical aspect for describing complex solid-state band structures. We show explicitly that the properties of the emitted fields are governed by the quantum statistics and quantum geometry of the underlying solid. Taking the Su-Schrieffer-Heeger (SSH) model in a one-sided optical cavity as a paradigmatic example and considering the dual regime, we demonstrate that in the topological phase a system exhibits a stronger HHG response and stronger quantum-light signatures than in the trivial phase. Furthermore, we show that cavity-matter interaction gives rise to squeezed high-harmonic quantum light, whose properties are directly imprinted by the current-current fluctuations in the material system. Crucially, the observed squeezing does not rely on a separate quartic Kerr mechanism. In the mesoscopic regime, the genuine quantum Kerr term is higher order in light-matter coupling strength and negligible, while the relevant non-classical effect is governed by current-current fluctuations encoded in the complex susceptibility of the material. This work establishes a direct link between band topology and photon statistics, opening new avenues for topology-sensitive quantum light generation and photon statistics based spectroscopy of solid-state systems.
| I am the presenting author | Yes |
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